Synthesis and investigation of the 5-formylcytidine modified, anticodon stem and loop of the human mitochondrial tRNAMet

نویسندگان

  • Hrvoje Lusic
  • Estella M. Gustilo
  • Franck A.P. Vendeix
  • Rob Kaiser
  • Michael O. Delaney
  • William D. Graham
  • Virginia A. Moye
  • William A. Cantara
  • Paul F. Agris
  • Alexander Deiters
چکیده

Human mitochondrial methionine transfer RNA (hmtRNA(Met)(CAU)) has a unique post-transcriptional modification, 5-formylcytidine, at the wobble position-34 (f(5)C(34)). The role of this modification in (hmtRNA(Met)(CAU)) for the decoding of AUA, as well as AUG, in both the peptidyl- and aminoacyl-sites of the ribosome in either chain initiation or chain elongation is still unknown. We report the first synthesis and analyses of the tRNA's anticodon stem and loop domain containing the 5-formylcytidine modification. The modification contributes to the tRNA's anticodon domain structure, thermodynamic properties and its ability to bind codons AUA and AUG in translational initiation and elongation.

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منابع مشابه

Synthesis and investigation of the 5-formylcytidine modified, anticodon stem and loop of the human mitochondrial tRNA

Human mitochondrial methionine transfer RNA ðhmtRNA CAUÞ has a unique post-transcriptional modification, 5-formylcytidine, at the wobble position-34 (fC34). The role of this modification in hmtRNA Met CAU for the decoding of AUA, as well as AUG, in both the peptidyland aminoacyl-sites of the ribosome in either chain initiation or chain elongation is still unknown. We report the first synthesis ...

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Unconventional decoding of the AUA codon as methionine by mitochondrial tRNAMet with the anticodon f5CAU as revealed with a mitochondrial in vitro translation system

Mitochondrial (mt) tRNA(Met) has the unusual modified nucleotide 5-formylcytidine (f(5)C) in the first position of the anticodon. This tRNA must translate both AUG and AUA as methionine. By constructing an in vitro translation system from bovine liver mitochondria, we examined the decoding properties of the native mt tRNA(Met) carrying f(5)C in the anticodon compared to a transcript that lacks ...

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Location alters tRNA identity: Trypanosoma brucei's cytosolic elongator tRNAMet is both the initiator and elongator in mitochondria.

A a rule, protein synthesis is initiated with methionine or formyl methionine from the first AUG codon in an ORF and that AUG is recognized by an initiator tRNAMet-i. Internal AUG codons are then translated by a second tRNA, the elongator tRNAMet-e (1). In eubacteria, mitochondria, and chloroplasts, the tRNAMet-i is charged with methionine, and subsequently the methionine is formylated by a met...

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NSUN3 and ABH1 modify the wobble position of mt‐tRNA Met to expand codon recognition in mitochondrial translation

Mitochondrial gene expression uses a non-universal genetic code in mammals. Besides reading the conventional AUG codon, mitochondrial (mt-)tRNAMet mediates incorporation of methionine on AUA and AUU codons during translation initiation and on AUA codons during elongation. We show that the RNA methyltransferase NSUN3 localises to mitochondria and interacts with mt-tRNAMet to methylate cytosine 3...

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Unconventional decoding of the AUA codon as methionine by mitochondrial tRNA with the anticodon fCAU as revealed with a mitochondrial in vitro translation system

Mitochondrial (mt) tRNA has the unusual modified nucleotide 5-formylcytidine (fC) in the first position of the anticodon. This tRNA must translate both AUG and AUA as methionine. By constructing an in vitro translation system from bovine liver mitochondria, we examined the decoding properties of the native mt tRNA carrying fC in the anticodon compared to a transcript that lacks the modification...

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عنوان ژورنال:

دوره 36  شماره 

صفحات  -

تاریخ انتشار 2008